Scientific Reports (Jun 2022)

Multiparameter laser performance characterization of liquid crystals for polarization control devices in the nanosecond regime

  • Kenneth L. Marshall,
  • Kyle R. P. Kafka,
  • Nathaniel D. Urban,
  • Jason U. Wallace,
  • Stavros G. Demos

DOI
https://doi.org/10.1038/s41598-022-14974-5
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 11

Abstract

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Abstract Interactions of liquid crystals (LC’s) with polarized light have been studied widely and have spawned numerous device applications, including the fabrication of optical elements for high-power and large-aperture laser systems. Currently, little is known about both the effect of incident polarization state on laser-induced–damage threshold (LIDT) and laser-induced functional threshold (LIFT) behavior at sub-LIDT fluences under multipulse irradiation conditions. This work reports on the first study of the nanosecond-pulsed LIDT’s dependence on incident polarization for several optical devices employing oriented nematic and chiral-nematic LC’s oriented by surface alignment layers. Accelerated lifetime testing was also performed to characterize the ability of these devices to maintain their functional performance under multipulse irradiation as a function of the laser fluence at both 1053 nm and 351 nm. Results show that the LIDT varies as a function of input polarization by 30–80% within the same device, while the multipulse LIFT (which can differ from the nominal LIDT) depends on irradiation conditions such as laser fluence and wavelength.