Mitigation of Membrane Fouling in Membrane Bioreactors Using Granular and Powdered Activated Carbon: An Experimental Study
Nataly Morales,
Camila Mery-Araya,
Paula Guerra,
Rodrigo Poblete,
Jaime Chacana-Olivares
Affiliations
Nataly Morales
Resource Recovery Laboratory, Faculty of Engineering and Geological Sciences, Department of Chemical and Environmental Engineering, Universidad Católica del Norte, 0610 Angamos Avenue, Antofagasta 1270709, Chile
Camila Mery-Araya
Department of Chemical and Environmental Engineering, Universidad Técnica Federico Santa María, 1680 España Avenue, Valparaíso 2390123, Chile
Paula Guerra
Department of Chemical and Environmental Engineering, Universidad Técnica Federico Santa María, 3939 Vicuña Mackenna Avenue, San Joaquín, Santiago 8940897, Chile
Rodrigo Poblete
Faculty of Marine Sciences, School of Risk Prevention and Environment, Universidad Católica del Norte, 1281 Larrondo, Coquimbo 1780000, Chile
Jaime Chacana-Olivares
Resource Recovery Laboratory, Faculty of Engineering and Geological Sciences, Department of Chemical and Environmental Engineering, Universidad Católica del Norte, 0610 Angamos Avenue, Antofagasta 1270709, Chile
This experimental study explores the mitigation of membrane fouling in membrane bioreactors (MBRs) through the combined use of granular activated carbon (GAC) and powdered activated carbon (PAC). The research assesses the impact of these materials on the fouling resistance, critical flux, and permeate quality using various mixed liquor suspended solids concentrations and carbon dosages. The results indicate that the GAC-PAC combination significantly reduces the total filtration resistance, particularly the cake layer resistance, by 11.7% to 13.6% compared to setups without activated carbon or with the individual carbon types. The study also reveals that this combination decreased the fouling rate by 15% to 24% at critical flux steps, demonstrating substantial improvements in fouling mitigation and operational efficiency. Furthermore, the GAC-PAC combination, which produces an adsorption process, enhances the permeate quality, achieving the near-complete removal of organic matter, total nitrogen, and turbidity, with total phosphorus removal reaching 99%. These findings demonstrate that the combined use of GAC and PAC not only reduces membrane fouling but also improves the overall MBR performance, making it a viable strategy for enhancing the efficiency of wastewater treatment processes.