Nature Communications (Apr 2024)

The nature of non-phononic excitations in disordered systems

  • Walter Schirmacher,
  • Matteo Paoluzzi,
  • Felix Cosmin Mocanu,
  • Dmytro Khomenko,
  • Grzegorz Szamel,
  • Francesco Zamponi,
  • Giancarlo Ruocco

DOI
https://doi.org/10.1038/s41467-024-46981-7
Journal volume & issue
Vol. 15, no. 1
pp. 1 – 16

Abstract

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Abstract The frequency scaling exponent of low-frequency excitations in microscopically small glasses, which do not allow for the existence of waves (phonons), has been in the focus of the recent literature. The density of states g(ω) of these modes obeys an ω s scaling, where the exponent s, ranging between 2 and 5, depends on the quenching protocol. The orgin of these findings remains controversal. Here we show, using heterogeneous-elasticity theory, that in a marginally-stable glass sample g(ω) follows a Debye-like scaling (s = 2), and the associated excitations (type-I) are of random-matrix type. Further, using a generalisation of the theory, we demonstrate that in more stable samples, other, (type-II) excitations prevail, which are non-irrotational oscillations, associated with local frozen-in stresses. The corresponding frequency scaling exponent s is governed by the statistics of small values of the stresses and, therefore, depends on the details of the interaction potential.