In the current work, a facile ion-solution spraying strategy was employed for one-step fabrication of CsPbBr3 perovskite thin films under atmosphere. The dependences of sample properties on annealing parameters (toleration temperature and duration time) were investigated in detail. As the results suggested, the sample prepared at 200 °C for 15 min featured better properties than others. The sample displayed a cubic phase with good crystallinity, a dense and compact morphology, a bandgap energy of 2.289 eV, and an average decay lifetime of 55.536 ns. Furthermore, the sample presented a Br-rich state, which was favorable for the carrier behavior and structure stability.
