Advanced Electronic Materials (Jul 2023)

Type‐II Dirac Nodal Lines in a Double‐Kagome‐Layered Semimetal

  • Yongqing Cai,
  • Jianfeng Wang,
  • Yuan Wang,
  • Zhanyang Hao,
  • Yixuan Liu,
  • Liang Zhou,
  • Xuelei Sui,
  • Zhicheng Jiang,
  • Shengjie Xu,
  • Han Ge,
  • Xiao‐Ming Ma,
  • Chengcheng Zhang,
  • Zecheng Shen,
  • Yichen Yang,
  • Qi Jiang,
  • Zhengtai Liu,
  • Mao Ye,
  • Dawei Shen,
  • Yi Liu,
  • Shengtao Cui,
  • Le Wang,
  • Cai Liu,
  • Junhao Lin,
  • Bing Huang,
  • Liusuo Wu,
  • Jincheng Zhuang,
  • Hongtao He,
  • Wenqing Zhang,
  • Jia‐Wei Mei,
  • Chaoyu Chen

DOI
https://doi.org/10.1002/aelm.202300212
Journal volume & issue
Vol. 9, no. 7
pp. n/a – n/a

Abstract

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Abstract Lorentz‐violating type‐II Dirac nodal line semimetals (DNLSs), hosting curves of band degeneracy formed by two dispersion branches with the same sign of slope, represent a novel state of matter. While being studied extensively in theory, convincing experimental evidence of type‐II DNLSs remain elusive. Recently, vanadium‐based kagome materials have emerged as a fertile ground to study the interplay between lattice symmetry and band topology. This work studies the low‐energy band structure of double‐kagome‐layered CsV8Sb12 and identifies it as a scarce type‐II DNLS protected by mirror symmetry. This work observes multiple DNLs consisting of type‐II Dirac cones close to or almost at the Fermi level via angle‐resolved photoemission spectroscopy (ARPES), which provides an electronic explanation for the nonsaturating magnetoresistance effect as observed. First‐principles theory analyses show that spin‐orbit coupling only opens a small gap, resulting in effectively gapless ARPES spectra, yet generating large spin Berry curvature. These type‐II DNLs, together with the interaction between a low‐energy van Hove singularity and quasi‐one‐dimensional band as observed in the same material, suggest CsV8Sb12 as an ideal platform for exploring novel transport properties.

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