Accelerating syngas-to-aromatic conversion via spontaneously monodispersed Fe in ZnCr2O4 spinel

Guo Tian; Xinyan Liu; Chenxi Zhang; Xiaoyu Fan; Hao Xiong; Xiao Chen; Zhengwen Li; Binhang Yan; Lan Zhang; Ning Wang; Hong-Jie Peng; Fei Wei

doi:10.1038/s41467-022-33217-9

Nature Communications (Sep 2022)

Accelerating syngas-to-aromatic conversion via spontaneously monodispersed Fe in ZnCr2O4 spinel

Guo Tian,
Xinyan Liu,
Chenxi Zhang,
Xiaoyu Fan,
Hao Xiong,
Xiao Chen,
Zhengwen Li,
Binhang Yan,
Lan Zhang,
Ning Wang,
Hong-Jie Peng,
Fei Wei

Affiliations

Guo Tian: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Xinyan Liu: Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China
Chenxi Zhang: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Xiaoyu Fan: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Hao Xiong: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Xiao Chen: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Zhengwen Li: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Binhang Yan: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University
Lan Zhang: Faculty of Environment and Life, Beijing University of Technology
Ning Wang: Faculty of Environment and Life, Beijing University of Technology
Hong-Jie Peng: Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China
Fei Wei: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University

DOI: https://doi.org/10.1038/s41467-022-33217-9
Journal volume & issue: Vol. 13, no. 1
pp. 1 – 11

Abstract

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Spontaneous monodispersion of active species and their stabilization in reductive atmospheres remain a challenge in catalytic syngas chemistry. Here the authors demonstrate that syngas-to-aromatic conversion can be significantly accelerated by the spontaneously monodispersed Fe in ZnCr2O4 spinel.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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