Second-order spectral lineshapes from charged interfaces

Paul E. Ohno; Hong-fei Wang; Franz M. Geiger

doi:10.1038/s41467-017-01088-0

Nature Communications (Oct 2017)

Second-order spectral lineshapes from charged interfaces

Paul E. Ohno,
Hong-fei Wang,
Franz M. Geiger

Affiliations

Paul E. Ohno: Department of Chemistry, Northwestern University
Hong-fei Wang: Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University
Franz M. Geiger: Department of Chemistry, Northwestern University

DOI: https://doi.org/10.1038/s41467-017-01088-0
Journal volume & issue: Vol. 8, no. 1
pp. 1 – 9

Abstract

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Charged interfaces are important in chemical systems, but the influence of charge on vibrational sum frequency spectra has only recently been considered. Here the authors show the importance of accounting for the interfacial potential-dependent χ(3) term in interpreting spectral lineshapes from charged interfaces.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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