npj Quantum Materials (Jun 2023)

Weak-coupling to strong-coupling quantum criticality crossover in a Kitaev quantum spin liquid α-RuCl3

  • Jae-Ho Han,
  • Seung-Hwan Do,
  • Kwang-Yong Choi,
  • Sang-Youn Park,
  • Jae-You Kim,
  • Sungdae Ji,
  • Ki-Seok Kim,
  • Jae-Hoon Park

DOI
https://doi.org/10.1038/s41535-023-00563-w
Journal volume & issue
Vol. 8, no. 1
pp. 1 – 12

Abstract

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Abstract We report a quantum criticality crossover representing two different universal scaling behaviors in a Kitaev quantum magnetic material α-RuCl3. α-RuCl3 presents both a symmetry-breaking antiferromagnetic order and a long-range entangled topological order of a quantum spin liquid, and thus could be a candidate system for a unique universality class involving deconfined fractionalized excitations of the local Z2 fluxes and itinerant Majorana fermions. Theoretical analyses on the inelastic neutron scattering, ac-magnetic susceptibility, and specific heat results demonstrate that Wilson–Fisher-Yukawa-type ‘conventional’ weak-coupling quantum criticality in high-energy scales crosses over to heavy-fermion-type ‘local’ strong-coupling one in low-energy scales. Our findings provide deep insight on how quantum criticality evolves in fermion-boson coupled topological systems with different types of deconfined fermions.