Chemical Engineering Journal Advances (Aug 2022)

Review and experimental comparison of the durability of iodine waste forms in semi-dynamic leach testing

  • Joelle T. Reiser,
  • Amanda R. Lawter,
  • Nancy A. Avalos,
  • Jeff Bonnett,
  • Brian J. Riley,
  • Saehwa Chong,
  • Nathan Canfield,
  • Sarah A. Saslow,
  • Agathe Bourchy,
  • R. Matthew Asmussen

Journal volume & issue
Vol. 11
p. 100300

Abstract

Read online

To ensure the safe disposal of radioiodine-containing nuclear wastes, a durable iodine waste form (IWF) is required. Many IWFs have been developed and evaluated for chemical durability using a wide range of test methods, making direct comparisons difficult as highlighted in this work through a review of available IWF corrosion data. To move toward a common dataset, a semi-dynamic leach test suite was experimentally demonstrated using several IWF types, providing standard comparisons. The results highlighted clear differences in corrosion resistance between various IWFs. This test suite is suggested for future studies to generate comparable data for a common dataset.

Keywords