Nature Communications (May 2021)

Combining density functional theory with macroscopic QED for quantum light-matter interactions in 2D materials

  • Mark Kamper Svendsen,
  • Yaniv Kurman,
  • Peter Schmidt,
  • Frank Koppens,
  • Ido Kaminer,
  • Kristian S. Thygesen

DOI
https://doi.org/10.1038/s41467-021-23012-3
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 13

Abstract

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The development of a quantitative and predictive theory of quantum light-matter interactions in ultrathin materials is both a conceptual and computational challenge. Here, the authors develop such a framework by combining density functional theory with macroscopic quantum electrodynamics, and use it to quantify the Purcell effect in van der Waals heterostructures.