npj Quantum Materials (May 2025)

One dimensional edge localized YSR states in CrCl3 on NbSe2

  • Jan P. Cuperus,
  • Arnold H. Kole,
  • Andrés R. Botello-Méndez,
  • Zeila Zanolli,
  • Daniel Vanmaekelbergh,
  • Ingmar Swart

DOI
https://doi.org/10.1038/s41535-025-00759-2
Journal volume & issue
Vol. 10, no. 1
pp. 1 – 6

Abstract

Read online

Abstract Magnet/superconductor hybrid systems have been put forward as a platform for realizing topological superconductivity. We investigated the heterostructure of ferromagnetic monolayer CrCl3 and superconducting NbSe2. Using low-temperature scanning tunneling microscopy, we observe topologically trivial Yu-Shiba-Rusinov (YSR) states localized at the edge of CrCl3 islands. DFT simulations reveal that the Cr atoms at the edge have an enhanced d-orbital DOS close to E F . This leads to an exchange coupling between these atoms and the substrate that rationalizes the edge-localization of the YSR states.