High repetition rate green-pumped supercontinuum generation in calcium fluoride

Abstract

Abstract We compare supercontinuum generation in $$\hbox {CaF}_2$$ CaF 2 crystal under tight and loose focusing of 150 fs, 515 nm second harmonic pulses from an amplified Yb:KGW laser at a repetition rate of 10 kHz. It is demonstrated that supercontinuum generation geometry applying loose focusing ( $$\hbox {NA}=0.004$$ NA = 0.004 ) of the pump beam into a long (25 mm) $$\hbox {CaF}_2$$ CaF 2 sample is advantageous in terms of supercontinuum spectral extent and durability of damage-free operation of the nonlinear material as compared to a commonly used supercontinuum generation setup which employs tight focusing ( $$\hbox {NA}=0.012$$ NA = 0.012 ) into a short (5 mm) sample and to setup which uses tight focusing into a long (25 mm) sample. More specifically, loose focusing into a long sample showed remarkably longer (20 min) damage-free operation of the nonlinear material, which was not translated with respect of the pump beam, while in tight focusing condition the sample is damaged just within 2 min of operation, leading to a complete extinction of the supercontinuum spectrum. The evolution of optical degradation of the nonlinear material in time and its impact to supercontinuum spectrum is studied in terms of filament-induced luminescence due to self-trapped exciton emission and light scattering at the pump wavelength indicating the onset of optical damage. Our findings are supported by the numerical simulations which compare relevant parameters related to filament propagation in tight and loose focusing conditions.