Physical Review Research (Feb 2023)

Characteristic length scales of the electrically induced insulator-to-metal transition

  • Theodor Luibrand,
  • Adrien Bercher,
  • Rodolfo Rocco,
  • Farnaz Tahouni-Bonab,
  • Lucia Varbaro,
  • Carl Willem Rischau,
  • Claribel Domínguez,
  • Yixi Zhou,
  • Weiwei Luo,
  • Soumen Bag,
  • Lorenzo Fratino,
  • Reinhold Kleiner,
  • Stefano Gariglio,
  • Dieter Koelle,
  • Jean-Marc Triscone,
  • Marcelo J. Rozenberg,
  • Alexey B. Kuzmenko,
  • Stefan Guénon,
  • Javier del Valle

DOI
https://doi.org/10.1103/PhysRevResearch.5.013108
Journal volume & issue
Vol. 5, no. 1
p. 013108

Abstract

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Some correlated materials display an insulator-to-metal transition as the temperature is increased. In most cases, this transition can also be induced electrically, resulting in volatile resistive switching due to the formation of a conducting filament. While this phenomenon has attracted much attention due to potential applications, many fundamental questions remain unaddressed. One of them is its characteristic lengths: What sets the size of these filaments, and how does this impact resistive switching properties? Here, we use a combination of wide-field and scattering-type scanning near-field optical microscopies to characterize filament formation in NdNiO_{3} and SmNiO_{3} thin films. We find a clear trend: Smaller filaments increase the current density, yielding sharper switching and a larger resistive drop. With the aid of numerical simulations, we discuss the parameters controlling the filament width and, hence, the switching properties.