Materials (Sep 2023)

Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers

  • Pao-Hsun Huang,
  • Sih-An Chen,
  • Li-Wei Chao,
  • Jia-Xun Xie,
  • Ching-Yu Liao,
  • Zong-Liang Tseng,
  • Sheng-Hui Chen

DOI
https://doi.org/10.3390/ma16176060
Journal volume & issue
Vol. 16, no. 17
p. 6060

Abstract

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Perovskite quantum dots (QDs) have showed excellent optoelectronic properties to extend the application range of novel solid-state lighting, such as perovskite QD based LEDs (QD-LEDs). However, the traditional device structure of perovskite QD-LEDs employed PEDOT:PSS as a hole inject layer (HIL), which impairs stability due to acidic surface characteristics. This study proposes the sputtered NiO films as an HIL to replace acidic PEDOT:PSS. The NiO films with significantly different characteristics were prepared by controlling the sputtering parameters to investigate the devices’ performance of NiO-based CsPbBr3 QD-LEDs. The optimized device showed an excellent performance with maxima luminescence of 20,118 cd/m2 and an external quantum efficiency (EQE) up to 3.63%.

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