Ultrafast Science (Jan 2024)

Spatial Aberrations in High-Order Harmonic Generation

  • Marius Plach,
  • Federico Vismarra,
  • Elisa Appi,
  • Vénus Poulain,
  • Jasper Peschel,
  • Peter Smorenburg,
  • David P. O’Dwyer,
  • Stephen Edward,
  • Yin Tao,
  • Rocío Borrego-Varillas,
  • Mauro Nisoli,
  • Cord L. Arnold,
  • Anne L’Huillier,
  • Per Eng-Johnsson

DOI
https://doi.org/10.34133/ultrafastscience.0054
Journal volume & issue
Vol. 4

Abstract

Read online

We investigate the spatial characteristics of high-order harmonic radiation generated in argon and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these patterns result from the order and generation position-dependent divergence of harmonics. Even small amounts of driving field astigmatism may result in cross-like patterns, coming from the superposition of individual harmonics with spatial profiles elongated in different directions. By correcting the aberrations using a deformable mirror, we show that fine-tuning the driving wavefront is essential for optimal spatial quality of the harmonics.