Solid Additive-Assisted Layer-by-Layer Processing for 19% Efficiency Binary Organic Solar Cells

Guanyu Ding; Tianyi Chen; Mengting Wang; Xinxin Xia; Chengliang He; Xiangjun Zheng; Yaokai Li; Di Zhou; Xinhui Lu; Lijian Zuo; Zhikang Xu; Hongzheng Chen

doi:10.1007/s40820-023-01057-x

Nano-Micro Letters (Apr 2023)

Solid Additive-Assisted Layer-by-Layer Processing for 19% Efficiency Binary Organic Solar Cells

Guanyu Ding,
Tianyi Chen,
Mengting Wang,
Xinxin Xia,
Chengliang He,
Xiangjun Zheng,
Yaokai Li,
Di Zhou,
Xinhui Lu,
Lijian Zuo,
Zhikang Xu,
Hongzheng Chen

Affiliations

Guanyu Ding: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Tianyi Chen: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Mengting Wang: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Xinxin Xia: Department of Physics, The Chinese University of Hong Kong
Chengliang He: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Xiangjun Zheng: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Yaokai Li: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Di Zhou: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University
Xinhui Lu: Department of Physics, The Chinese University of Hong Kong
Lijian Zuo: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University
Zhikang Xu: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University
Hongzheng Chen: State Key Laboratory of Silicon Materials, Department of Polymer Science and Engineering, Zhejiang University

DOI: https://doi.org/10.1007/s40820-023-01057-x
Journal volume & issue: Vol. 15, no. 1
pp. 1 – 14

Abstract

Read online

Highlights A solid additive-assisted layer-by-layer (SAA-LBL) processing was developed to facilitate the inter-diffusion between polymer donor and acceptor and optimize the morphology of quasi-planar heterojunction for high-performance organic solar cells (OSCs). The pre-phase separation between fatty acid and polymer donor, easily tuned via controlling the cohesive energy, is critical to form the desired vertical phase-separation morphology. The SAA-LBL is generally applicable to various OSC systems, and enables the record efficiency of 19.02% among the binary OSCs.

Published in Nano-Micro Letters

ISSN: 2311-6706 (Print); 2150-5551 (Online)
Publisher: SpringerOpen
Country of publisher: Germany
LCC subjects: Technology
Website: http://www.springer.com/40820

About the journal

Abstract

Keywords