In this article, water-based polyurethane (PU) with different concentrations and partial alcoholysis polyvinyl alcohol (PVA) were used to coat polyester (PET) harness cord in turn. The surface and mechanical properties of harness cord before and after coating were evaluated by performing the tests of dynamic contact angle, morphology observation, bending properties, tensile properties, and wearability. It was found that the surface properties of 1.5% PU-coated harness cord tended to be stable, and the mechanical properties of PU(1.5%)/PVA-coated harness cord were optimal. Compared with PVA-coated harness cord, the wearability of PU(1.5%)/PVA-coated harness cord showed a great increment up to 135.7%. This was because the PU coating effectively improved the interfacial properties between the PVA coating and the hydrophobic PET fibers and enhanced the adhesion of the PVA coating to the PET fibers.
