Superimposed effects of typical local circulations driven by mountainous topography and aerosol–radiation interaction on heavy haze in the Beijing–Tianjin–Hebei central and southern plains in winter

Abstract

Although China's air quality has substantially improved in recent years due to the vigorous emissions reduction, the Beijing–Tianjin–Hebei (BTH) region, especially its central and southern plains at the eastern foot of the Taihang Mountains, has been the most polluted area in China, with persistent and severe haze in winter. Combining meteorology–chemistry coupled model simulations and multiple observations, this study explored the causes of several heavy haze events in this area in January 2017, focusing on local circulations related to mountain terrain. The study results showed that on the weather scale, the configuration of the upper, middle, and lower atmosphere provided favorable weather and water vapor transport conditions for the development of haze pollution. Under the weak weather-scale systems, local circulation played a dominant role in the regional distribution and extreme values of PM2.5. Influenced by the Taihang and Yanshan mountains, vertical circulations and wind convergence zone were formed between the plain and mountain slopes. The vertical distribution of pollutants strongly depended on the intensity and location of the circulation. The circulation with high intensity and low altitude was more unfavorable for the vertical and horizontal diffusion of near-surface pollutants. More importantly, we found that the aerosol–radiation interaction (ARI) significantly amplified the impacts of local vertical circulations on heavy haze by two mechanisms. First, the ARI strengthened the vertical circulations at the lower levels, with the zonal wind speeds increasing by 0.3–0.8 m s−1. Meanwhile, the ARI could cause a substantial downward shift in the vertical circulations (∼ 100 m). Second, the ARI weakened the horizontal diffusion of pollutants by reducing the westerly winds and enhancing wind convergence and southerly winds. Under these two mechanisms, pollutants could only recirculate in a limited space. This superposition of the typical local circulation and the ARI eventually contributed to the accumulation of pollutants and the consequent deterioration of haze pollution in the region.