Nature Communications (Jun 2021)

Are Shockley-Read-Hall and ABC models valid for lead halide perovskites?

  • Alexander Kiligaridis,
  • Pavel A. Frantsuzov,
  • Aymen Yangui,
  • Sudipta Seth,
  • Jun Li,
  • Qingzhi An,
  • Yana Vaynzof,
  • Ivan G. Scheblykin

DOI
https://doi.org/10.1038/s41467-021-23275-w
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 13

Abstract

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Charge dynamics in perovskite is not well-understood, limited by the knowledge of defect physics and charge recombination mechanism, yet the ABC and SRH models are widely used. Here, the authors introduce advanced PLQY mapping as function of excitation pulse energy and repetition frequency to examine the validity of these models.