Nature Communications (Jul 2024)

Strong angular and spectral narrowing of electroluminescence in an integrated Tamm-plasmon-driven halide perovskite LED

  • Zher Ying Ooi,
  • Alberto Jiménez-Solano,
  • Krzysztof Gałkowski,
  • Yuqi Sun,
  • Jordi Ferrer Orri,
  • Kyle Frohna,
  • Hayden Salway,
  • Simon Kahmann,
  • Shenyu Nie,
  • Guadalupe Vega,
  • Shaoni Kar,
  • Michał P. Nowak,
  • Sebastian Maćkowski,
  • Piotr Nyga,
  • Caterina Ducati,
  • Neil C. Greenham,
  • Bettina V. Lotsch,
  • Miguel Anaya,
  • Samuel D. Stranks

DOI
https://doi.org/10.1038/s41467-024-49838-1
Journal volume & issue
Vol. 15, no. 1
pp. 1 – 10

Abstract

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Abstract Next-generation light-emitting applications such as displays and optical communications require judicious control over emitted light, including intensity and angular dispersion. To date, this remains a challenge as conventional methods require cumbersome optics. Here, we report highly directional and enhanced electroluminescence from a solution-processed quasi-2-dimensional halide perovskite light-emitting diode by building a device architecture to exploit hybrid plasmonic-photonic Tamm plasmon modes. By exploiting the processing and bandgap tunability of the halide perovskite device layers, we construct the device stack to optimise both optical and charge-injection properties, leading to narrow forward electroluminescence with an angular full-width half-maximum of 36.6° compared with the conventional isotropic control device of 143.9°, and narrow electroluminescence spectral full-width half-maximum of 12.1 nm. The device design is versatile and tunable to work with emission lines covering the visible spectrum with desired directionality, thus providing a promising route to modular, inexpensive, and directional operating light-emitting devices.