Materials Research Letters (Feb 2024)

Thermoelectric performance of SnTe nano-films depending on thickness, doping concentration and temperature

  • Jie Zhu,
  • Xuanhui Fan,
  • Kewen Zhang,
  • Jing Zhou,
  • Dawei Tang

DOI
https://doi.org/10.1080/21663831.2024.2307372
Journal volume & issue
Vol. 12, no. 2
pp. 140 – 147

Abstract

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Tin telluride (SnTe), a promising mid-temperature thermoelectric material, faces limitations due to inherent vacancies and band characteristics. Low-dimensionalization represents one avenue to potentially improve thermoelectric performance. This work explores the SnTe films with varying thicknesses (67–610 nm) and Zn doping concentration (0–12.81%) at high temperature. A 224 nm-SnTe-film exhibits optimal ZT values (0.27 at 600 K), and the Zn-doped films experience impaired thermoelectric properties, with the electrical conductivity reduction being a primary contributor. This study contributes valuable insights for enhancing thin-film SnTe's thermoelectric performance and developing eco-friendly mid-temperature thermoelectric materials.

Keywords