Scientific Reports (Dec 2022)

Photon extraction enhancement of praseodymium ions in gallium nitride nanopillars

  • Shin-ichiro Sato,
  • Shuo Li,
  • Andrew D. Greentree,
  • Manato Deki,
  • Tomoaki Nishimura,
  • Hirotaka Watanabe,
  • Shugo Nitta,
  • Yoshio Honda,
  • Hiroshi Amano,
  • Brant C. Gibson,
  • Takeshi Ohshima

DOI
https://doi.org/10.1038/s41598-022-25522-6
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 11

Abstract

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Abstract Lanthanoid-doped Gallium Nitride (GaN) integrated into nanophotonic technologies is a promising candidate for room-temperature quantum photon sources for quantum technology applications. We manufactured praseodymium (Pr)-doped GaN nanopillars of varying size, and showed significantly enhanced room-temperature photon extraction efficiency compared to unstructured Pr-doped GaN. Implanted Pr ions in GaN show two main emission peaks at 650.3 nm and 651.8 nm which are attributed to 3 P 0-3 F 2 transition in the 4f-shell. The maximum observed enhancement ratio was 23.5 for 200 nm diameter circular pillars, which can be divided into the emitted photon extraction enhancement by a factor of 4.5 and the photon collection enhancement by a factor of 5.2. The enhancement mechanism is explained by the eigenmode resonance inside the nanopillar. Our study provides a pathway for Lanthanoid-doped GaN nano/micro-scale photon emitters and quantum technology applications.