The gel-state grease plays a vital and indispensable role in the long-term operation of wind turbines. To reduce carbon emissions and increase the reliability of wind turbines, this paper takes the gel-state Mobil SHC 461WT grease as the study object. Firstly, the rheological properties of the gel-state Mobil SHC 461WT grease were investigated using the Anton Paar MCR302 rotational rheometer. Secondly, the rheological characteristics of three different gel states of the Mobil SHC 461WT grease (additive content of 0.1% of RFM3000, SK3115, and PV611, respectively, in the gel-state Mobil SHC 461WT grease) were optimized under the same conditions. Finally, according to the experimental results and the Herschel–Bulkley (H–B) model, the RFM3000 additive has the best effect on improving the rheological characteristics of the gel-state Mobil SHC 461WT grease. This research provides a new idea and direction for the technological advancement of the gel-state grease industry.