Non-classical light scattered by laser-pumped molecules possessing permanent dipoles

Abstract

Squeezing in resonance fluorescence processes of a laser-pumped molecule possessing permanent dipoles is shown. A weak low-frequency coherent field pumps the sample near resonance with the dynamically Stark-splitting states induced by a second stronger laser field driving the main two-level transition. The fluorescence spectrum consists of three coherently scattered spectral lines and up to nine incoherently scattered spectral lines. Compared with a similar problem yet in the absence of permanent dipoles, aditional squeezing regions are found.