Instrumental characteristics and potential greenhouse gas measurement capabilities of the Compact High-Spectral-Resolution Infrared Spectrometer: CHRIS

Abstract

Ground-based high-spectral-resolution infrared measurements are an efficient way to obtain accurate tropospheric abundances of different gaseous species, in particular greenhouse gases (GHGs) such as CO2 and CH4. Many ground-based spectrometers are used in the NDACC and TCCON networks to validate the Level 2 satellite data, but their large dimensions and heavy mass make them inadequate for field campaigns. To overcome these problems, the use of portable spectrometers was recently investigated. In this context, this paper deals with the CHRIS (Compact High-Spectral-Resolution Infrared Spectrometer) prototype with unique characteristics such as its high spectral resolution (0.135 cm−1 nonapodized) and its wide spectral range (680 to 5200 cm−1). Its main objective is the characterization of gases and aerosols in the thermal and shortwave infrared regions. That is why it requires high radiometric precision and accuracy, which are achieved by performing spectral and radiometric calibrations that are described in this paper. Furthermore, CHRIS's capabilities to retrieve vertical CO2 and CH4 profiles are presented through a complete information content analysis, a channel selection and an error budget estimation in the attempt to join ongoing campaigns such as MAGIC (Monitoring of Atmospheric composition and Greenhouse gases through multi-Instruments Campaigns) to monitor GHGs and validate the actual and future space missions such as IASI-NG and Microcarb.