Physical Review X (Aug 2016)

Ultracold Chemical Reactions of a Single Rydberg Atom in a Dense Gas

  • Michael Schlagmüller,
  • Tara Cubel Liebisch,
  • Felix Engel,
  • Kathrin S. Kleinbach,
  • Fabian Böttcher,
  • Udo Hermann,
  • Karl M. Westphal,
  • Anita Gaj,
  • Robert Löw,
  • Sebastian Hofferberth,
  • Tilman Pfau,
  • Jesús Pérez-Ríos,
  • Chris H. Greene

DOI
https://doi.org/10.1103/PhysRevX.6.031020
Journal volume & issue
Vol. 6, no. 3
p. 031020

Abstract

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Within a dense environment (ρ≈10^{14} atoms/cm^{3}) at ultracold temperatures (T140 compared to 1 μs at n=90. In addition, a second observed reaction mechanism, namely, Rb_{2}^{+} molecule formation, was studied. Both reaction products are equally probable for n=40, but the fraction of Rb_{2}^{+} created drops to below 10% for n≥90.