Nature Communications (Feb 2023)

Steering carbon dioxide reduction toward C–C coupling using copper electrodes modified with porous molecular films

  • Siqi Zhao,
  • Oliver Christensen,
  • Zhaozong Sun,
  • Hongqing Liang,
  • Alexander Bagger,
  • Kristian Torbensen,
  • Pegah Nazari,
  • Jeppe Vang Lauritsen,
  • Steen Uttrup Pedersen,
  • Jan Rossmeisl,
  • Kim Daasbjerg

DOI
https://doi.org/10.1038/s41467-023-36530-z
Journal volume & issue
Vol. 14, no. 1
pp. 1 – 11

Abstract

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This study explores how the activity and selectivity of Cu electrodes for CO2 reduction can be tuned with organic films of different porosity and thickness. As a result, the films increase the local CO partial pressures and surface coverages.