Nature Communications (Apr 2022)
Enabling high energy lithium metal batteries via single-crystal Ni-rich cathode material co-doping strategy
- Xing Ou,
- Tongchao Liu,
- Wentao Zhong,
- Xinming Fan,
- Xueyi Guo,
- Xiaojing Huang,
- Liang Cao,
- Junhua Hu,
- Bao Zhang,
- Yong S. Chu,
- Guorong Hu,
- Zhang Lin,
- Mouad Dahbi,
- Jones Alami,
- Khalil Amine,
- Chenghao Yang,
- Jun Lu
Affiliations
- Xing Ou
- Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, School of Environment and Energy, South China University of Technology
- Tongchao Liu
- Chemical Sciences and Engineering Division, Argonne National Laboratory
- Wentao Zhong
- Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, School of Environment and Energy, South China University of Technology
- Xinming Fan
- School of Metallurgy and Environment, Central South University
- Xueyi Guo
- School of Metallurgy and Environment, Central South University
- Xiaojing Huang
- National Synchrotron Light source II, Brookhaven National Laboratory
- Liang Cao
- Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, School of Environment and Energy, South China University of Technology
- Junhua Hu
- School of Materials Science and Engineering, Zhengzhou University
- Bao Zhang
- School of Metallurgy and Environment, Central South University
- Yong S. Chu
- National Synchrotron Light source II, Brookhaven National Laboratory
- Guorong Hu
- School of Metallurgy and Environment, Central South University
- Zhang Lin
- School of Metallurgy and Environment, Central South University
- Mouad Dahbi
- Materials Science and Nano-Engineering Department, Mohammed VI Polytechnic University
- Jones Alami
- Materials Science and Nano-Engineering Department, Mohammed VI Polytechnic University
- Khalil Amine
- Chemical Sciences and Engineering Division, Argonne National Laboratory
- Chenghao Yang
- Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, School of Environment and Energy, South China University of Technology
- Jun Lu
- Chemical Sciences and Engineering Division, Argonne National Laboratory
- DOI
- https://doi.org/10.1038/s41467-022-30020-4
- Journal volume & issue
-
Vol. 13,
no. 1
pp. 1 – 12
Abstract
Li-ion cathode active materials are transitioning from poly- to single-crystal structures. However, the performance of high Ni-content single-crystal cathodes remains below expectations. Here, via Al/Zr co-doping, the authors propose a strategy to mitigate structural degradation in this class of materials.
