Physical Review Research (Jun 2021)

Long-time diffusion and energy transfer in polydisperse mixtures of particles with different temperatures

  • Efe Ilker,
  • Michele Castellana,
  • Jean-François Joanny

DOI
https://doi.org/10.1103/PhysRevResearch.3.023207
Journal volume & issue
Vol. 3, no. 2
p. 023207

Abstract

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Evidence suggests that the transport rate of a passive particle at long time scales is enhanced due to interactions with the surrounding active ones in a size- and composition-dependent manner. Using a system of particles with different temperatures, we probe these effects in dilute solutions and derive long-time friction and self-diffusion coefficients as functions of volume fractions, sizes, and temperatures of particles in d=2 and 3 dimensions. Thus, we model excluded-volume interactions for nonequilibrium systems but also extend the scope to short-range soft potentials and compare our results to Brownian-dynamics simulations. Remarkably, we show that both viscosity and energy flux display a nonlinear dependence on size. The simplicity of our formalism allows to discover various interesting scenarios that can be relevant for biological systems and active colloids.