Phase-matched five-wave mixing in zinc oxide microwire
Cui Kaibo,
Zhang Tianzhu,
Rao Tao,
Zhang Xianghui,
Zhang Shunping,
Xu Hongxing
Affiliations
Cui Kaibo
School of Physics and Technology and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan University12390, Wuhan430072, China
Zhang Tianzhu
School of Physics and Technology and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan University12390, Wuhan430072, China
Rao Tao
Hubei Key Laboratory of Micro-Nanoelectronic Materials and Devices, School of Microelectronics, Hubei University, Wuhan430062, China
Zhang Xianghui
Hubei Key Laboratory of Micro-Nanoelectronic Materials and Devices, School of Microelectronics, Hubei University, Wuhan430062, China
Zhang Shunping
School of Physics and Technology and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan University12390, Wuhan430072, China
Xu Hongxing
School of Physics and Technology and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan University12390, Wuhan430072, China
High-order wave mixing in solid-state platforms gather increasing importance due to the development of advanced lasers and integrated photonic circuit for both classical and quantum information. However, the high-order wave mixing is generally inefficient in solids under weak pump. Here, we observed the presence of phase matching of five-wave mixing (5WM) propagating in a zinc oxide (ZnO) microwire. The 5WM signal is enhanced by 2–3 orders of magnitude under the phase matching conditions, reaching an absolute conversion efficiency of 1.7 × 10−13 when the peak pumping power density is about 106 W/cm2. The propagation of multiple nonlinear signals, including sum frequency generation, third harmonic generation, four-wave mixing etc., benefited from both the large nonlinear coefficients and the wide transparent window of ZnO, implies the possibility of developing cascaded nonlinear process under higher pumping. This study enriches the ZnO platform for integrated nonlinear nanophotonics.