Balancing hydrogen adsorption/desorption by orbital modulation for efficient hydrogen evolution catalysis

Feng Li; Gao-Feng Han; Hyuk-Jun Noh; Jong-Pil Jeon; Ishfaq Ahmad; Shanshan Chen; Changduk Yang; Yunfei Bu; Zhengping Fu; Yalin Lu; Jong-Beom Baek

doi:10.1038/s41467-019-12012-z

Nature Communications (Sep 2019)

Balancing hydrogen adsorption/desorption by orbital modulation for efficient hydrogen evolution catalysis

Feng Li,
Gao-Feng Han,
Hyuk-Jun Noh,
Jong-Pil Jeon,
Ishfaq Ahmad,
Shanshan Chen,
Changduk Yang,
Yunfei Bu,
Zhengping Fu,
Yalin Lu,
Jong-Beom Baek

Affiliations

Feng Li: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)
Gao-Feng Han: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)
Hyuk-Jun Noh: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)
Jong-Pil Jeon: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)
Ishfaq Ahmad: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)
Shanshan Chen: MOE Key Laboratory of Low-grade Energy Utilization Technologies and Systems, CQU-NUS Renewable Energy Materials & Devices Joint Laboratory, School of Energy & Power Engineering, Chongqing University
Changduk Yang: Department of Energy Engineering, School of Energy and Chemical Engineering, Perovtronics Research Center, Low Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST)
Yunfei Bu: School of Environmental Science and Engineering, Nanjing University of Information Science and Technology
Zhengping Fu: CAS Key Laboratory of Materials for Energy Conversion, Hefei National Laboratory for Physical Sciences at Microscale, National Synchrotron Radiation Laboratory, University of Science and Technology of China
Yalin Lu: CAS Key Laboratory of Materials for Energy Conversion, Hefei National Laboratory for Physical Sciences at Microscale, National Synchrotron Radiation Laboratory, University of Science and Technology of China
Jong-Beom Baek: School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST)

DOI: https://doi.org/10.1038/s41467-019-12012-z
Journal volume & issue: Vol. 10, no. 1
pp. 1 – 7

Abstract

Read online

Hydrogen adsorption/desorption behavior plays a key role in hydrogen evolution reaction catalysis. Here, the authors demonstrate the rational balancing of hydrogen adsorption/desorption by orbital modulation for significantly enhanced hydrogen evolution performance.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

About the journal