Nature Communications (Nov 2022)
Fine-tuned local coordination environment of Pt single atoms on ceria controls catalytic reactivity
- Wei Tan,
- Shaohua Xie,
- Duy Le,
- Weijian Diao,
- Meiyu Wang,
- Ke-Bin Low,
- Dave Austin,
- Sampyo Hong,
- Fei Gao,
- Lin Dong,
- Lu Ma,
- Steven N. Ehrlich,
- Talat S. Rahman,
- Fudong Liu
Affiliations
- Wei Tan
- Department of Civil, Environmental, and Construction Engineering, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), NanoScience Technology Center (NSTC), University of Central Florida
- Shaohua Xie
- Department of Civil, Environmental, and Construction Engineering, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), NanoScience Technology Center (NSTC), University of Central Florida
- Duy Le
- Department of Physics, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), University of Central Florida
- Weijian Diao
- Department of Chemical and Biological Engineering, Villanova University
- Meiyu Wang
- College of Engineering and Applied Sciences, Nanjing University
- Ke-Bin Low
- BASF Corporation
- Dave Austin
- Department of Physics, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), University of Central Florida
- Sampyo Hong
- Brewton-Parker College
- Fei Gao
- State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment; Jiangsu Key Laboratory of Vehicle Emissions Control, School of Chemistry and Chemical Engineering; Center of Modern Analysis, Nanjing University
- Lin Dong
- State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment; Jiangsu Key Laboratory of Vehicle Emissions Control, School of Chemistry and Chemical Engineering; Center of Modern Analysis, Nanjing University
- Lu Ma
- National Synchrotron Light Source II (NSLS-II), Brookhaven National Laboratory
- Steven N. Ehrlich
- National Synchrotron Light Source II (NSLS-II), Brookhaven National Laboratory
- Talat S. Rahman
- Department of Physics, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), University of Central Florida
- Fudong Liu
- Department of Civil, Environmental, and Construction Engineering, Catalysis Cluster for Renewable Energy and Chemical Transformations (REACT), NanoScience Technology Center (NSTC), University of Central Florida
- DOI
- https://doi.org/10.1038/s41467-022-34797-2
- Journal volume & issue
-
Vol. 13,
no. 1
pp. 1 – 16
Abstract
CeO2-supported Pt single atoms with different coordination environments exhibit distinct behaviors in reactant adsorption/activation and product desorption, thus showing different catalytic performance for various catalytic oxidation reactions.
