Nanomaterials (Jan 2023)

Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure

  • Zijie Ji,
  • Ruan Zhang,
  • Shuangxing Zhu,
  • Feifan Gu,
  • Yunmin Jin,
  • Binghe Xie,
  • Jiaxin Wu,
  • Xinghan Cai

DOI
https://doi.org/10.3390/nano13030421
Journal volume & issue
Vol. 13, no. 3
p. 421

Abstract

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The photo-induced superconducting phase transition is widely used in probing the physical properties of correlated electronic systems and to realize broadband photodetection with extremely high responsivity. However, such photoresponse is usually insensitive to electrostatic doping due to the high carrier density of the superconductor, restricting its applications in tunable optoelectronic devices. In this work, we demonstrate the gate voltage modulation to the photoresponsivity in a two-dimensional NbSe2-graphene heterojunction. The superconducting critical current of the NbSe2 relies on the gate-dependent hot carrier generation in graphene via the Joule heating effect, leading to the observed shift of both the magnitude and peak position of the photoresponsivity spectra as the gate voltage changes. This heating effect is further confirmed by the temperature and laser-power-dependent characterization of the photoresponse. In addition, we investigate the spatially-resolved photocurrent, finding that the superconductivity is inhomogeneous across the junction area. Our results provide a new platform for designing tunable superconducting photodetector and indicate that the photoresponse could be a powerful tool in studying the local electronic properties and phase transitions in low-dimensional superconducting systems.

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