Nature Communications (Sep 2020)
Atomically-precise dopant-controlled single cluster catalysis for electrochemical nitrogen reduction
- Chuanhao Yao,
- Na Guo,
- Shibo Xi,
- Cong-Qiao Xu,
- Wei Liu,
- Xiaoxu Zhao,
- Jing Li,
- Hanyan Fang,
- Jie Su,
- Zhongxin Chen,
- Huan Yan,
- Zhizhan Qiu,
- Pin Lyu,
- Cheng Chen,
- Haomin Xu,
- Xinnan Peng,
- Xinzhe Li,
- Bin Liu,
- Chenliang Su,
- Stephen J. Pennycook,
- Cheng-Jun Sun,
- Jun Li,
- Chun Zhang,
- Yonghua Du,
- Jiong Lu
Affiliations
- Chuanhao Yao
- Department of Chemistry, National University of Singapore
- Na Guo
- Department of Physics, National University of Singapore
- Shibo Xi
- Institute of Chemical and Engineering Sciences
- Cong-Qiao Xu
- Department of Chemistry, Southern University of Science and Technology
- Wei Liu
- Department of Chemistry, National University of Singapore
- Xiaoxu Zhao
- Department of Chemistry, National University of Singapore
- Jing Li
- Department of Chemistry, National University of Singapore
- Hanyan Fang
- Department of Chemistry, National University of Singapore
- Jie Su
- Department of Chemistry, National University of Singapore
- Zhongxin Chen
- Department of Chemistry, National University of Singapore
- Huan Yan
- Department of Chemistry, National University of Singapore
- Zhizhan Qiu
- Department of Chemistry, National University of Singapore
- Pin Lyu
- Department of Chemistry, National University of Singapore
- Cheng Chen
- Department of Chemistry, National University of Singapore
- Haomin Xu
- Department of Chemistry, National University of Singapore
- Xinnan Peng
- Department of Chemistry, National University of Singapore
- Xinzhe Li
- Department of Chemistry, National University of Singapore
- Bin Liu
- School of Chemical and Biomedical Engineering, Nanyang Technological University
- Chenliang Su
- SZU-NUS Collaborative Centre and International Collaborative Laboratory of 2D Materials for Optoelectronic Science & Technology, College of Optoelectronic Engineering, Shenzhen University
- Stephen J. Pennycook
- NUS Graduate School for Integrative Sciences and Engineering, National University of Singapore
- Cheng-Jun Sun
- Advanced Photon Source, Argonne National Laboratory
- Jun Li
- Department of Chemistry, Southern University of Science and Technology
- Chun Zhang
- Department of Chemistry, National University of Singapore
- Yonghua Du
- Institute of Chemical and Engineering Sciences
- Jiong Lu
- Department of Chemistry, National University of Singapore
- DOI
- https://doi.org/10.1038/s41467-020-18080-w
- Journal volume & issue
-
Vol. 11,
no. 1
pp. 1 – 10
Abstract
The fabrication of singly dispersed metal cluster catalysts with atomic-level control of dopants is a long-standing challenge. Here, the authors report a strategy for the synthesis of a precisely doped single cluster catalyst which shows exceptional activity for electrochemical dinitrogen reduction.