Complex interplay of sulfate aerosols and meteorology conditions on precipitation and latent heat vertical structure

Abstract

Abstract An eight-year satellite observation dataset reveals that sulfate aerosols significantly influence the vertical structure of precipitation and latent heat (LH) in the Beijing-Tianjin-Hebei (BTH) region during summer. In this period, prevalent sulfate aerosols combine with warm, humid southerly winds and elevated convective available potential energy (CAPE), influencing precipitation dynamics. Under polluted conditions with specific CAPE and precipitation top temperature (PTT) ranges, precipitation particles experience accelerated growth within the mixed-phase layer, delineated by the −5 °C to 2 °C isotherms, compared to pristine environments. This results in a marked increase in both the intensity and height at which the maximum LH is released. Subsequent analysis reveals that hygroscopic sulfate aerosols, acting as cloud condensation nuclei (CCN), amplify the collision-coalescence process within the mixed layer amid high cloud water content, propelling rapid precipitation particle growth and elevating the PTT. This warming effect surpasses the cooling contribution from robust CAPE, culminating in a net elevation of PTT under polluted scenarios compared to pristine ones. Additionally, quantification of PTT sensitivity to both CAPE and aerosol optical depth (AOD) unveils a high consistency between satellite-detected PTT responses to CAPE and those predicted by cloud-resolving model simulations. The study deduces that the role of aerosols as CCN in either invigorating or diminishing the collision-coalescence process is contingent on the available cloud water.