Electrical Properties and Strain Sensing Mechanisms in Hybrid Graphene Nanoplatelet/Carbon Nanotube Nanocomposites
Xoan F. Sánchez-Romate,
Alberto Jiménez-Suárez,
Mónica Campo,
Alejandro Ureña,
Silvia G. Prolongo
Affiliations
Xoan F. Sánchez-Romate
Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnología, Universidad Rey Juan Carlos, Calle Tulipán s/n, Móstoles, 28933 Madrid, Spain
Alberto Jiménez-Suárez
Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnología, Universidad Rey Juan Carlos, Calle Tulipán s/n, Móstoles, 28933 Madrid, Spain
Mónica Campo
Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnología, Universidad Rey Juan Carlos, Calle Tulipán s/n, Móstoles, 28933 Madrid, Spain
Alejandro Ureña
Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnología, Universidad Rey Juan Carlos, Calle Tulipán s/n, Móstoles, 28933 Madrid, Spain
Silvia G. Prolongo
Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnología, Universidad Rey Juan Carlos, Calle Tulipán s/n, Móstoles, 28933 Madrid, Spain
Electrical and electromechanical properties of hybrid graphene nanoplatelet (GNP)/carbon nanotube (CNT)-reinforced composites were analyzed under two different sonication conditions. The electrical conductivity increases with increasing nanofiller content, while the optimum sonication time decreases in a low viscosity media. Therefore, for samples with a higher concentration of GNPs, an increase of sonication time of the hybrid GNP/CNT mixture generally leads to an enhancement of the electrical conductivity, up to values of 3 S/m. This means that the optimum sonication process to achieve the best performances is reached in the longest times. Strain sensing tests show a higher prevalence of GNPs at samples with a high GNP/CNT ratio, reaching gauge factors of around 10, with an exponential behavior of electrical resistance with applied strain, whereas samples with lower GNP/CNT ratio have a more linear response owing to a higher prevalence of CNT tunneling transport mechanisms, with gauge factors of around 3–4.