Promoting ethylene production over a wide potential window on Cu crystallites induced and stabilized via current shock and charge delocalization

Hao Sun; Ling Chen; Likun Xiong; Kun Feng; Yufeng Chen; Xiang Zhang; Xuzhou Yuan; Baiyu Yang; Zhao Deng; Yu Liu; Mark H. Rümmeli; Jun Zhong; Yan Jiao; Yang Peng

doi:10.1038/s41467-021-27169-9

Nature Communications (Nov 2021)

Promoting ethylene production over a wide potential window on Cu crystallites induced and stabilized via current shock and charge delocalization

Hao Sun,
Ling Chen,
Likun Xiong,
Kun Feng,
Yufeng Chen,
Xiang Zhang,
Xuzhou Yuan,
Baiyu Yang,
Zhao Deng,
Yu Liu,
Mark H. Rümmeli,
Jun Zhong,
Yan Jiao,
Yang Peng

Affiliations

Hao Sun: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Ling Chen: School of Chemical Engineering and Advanced Materials, The University of Adelaide
Likun Xiong: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Kun Feng: Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University
Yufeng Chen: Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University
Xiang Zhang: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Xuzhou Yuan: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Baiyu Yang: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Zhao Deng: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Yu Liu: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Mark H. Rümmeli: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University
Jun Zhong: Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University
Yan Jiao: School of Chemical Engineering and Advanced Materials, The University of Adelaide
Yang Peng: Soochow Institute for Energy and Materials Innovations, College of Energy, Soochow University

DOI: https://doi.org/10.1038/s41467-021-27169-9
Journal volume & issue: Vol. 12, no. 1
pp. 1 – 11

Abstract

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The substrate-catalyst interaction plays a critical role in steering the pathway of electrochemical CO2 reduction. Here the authors show the crystalline states of copper in reconstructed metal-organic frameworks were induced and stabilized by Ketjen Black conducting support, promoting C2H4 production.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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