Nature Communications (Mar 2021)

Dynamic lattice distortions driven by surface trapping in semiconductor nanocrystals

  • Burak Guzelturk,
  • Benjamin L. Cotts,
  • Dipti Jasrasaria,
  • John P. Philbin,
  • David A. Hanifi,
  • Brent A. Koscher,
  • Arunima D. Balan,
  • Ethan Curling,
  • Marc Zajac,
  • Suji Park,
  • Nuri Yazdani,
  • Clara Nyby,
  • Vladislav Kamysbayev,
  • Stefan Fischer,
  • Zach Nett,
  • Xiaozhe Shen,
  • Michael E. Kozina,
  • Ming-Fu Lin,
  • Alexander H. Reid,
  • Stephen P. Weathersby,
  • Richard D. Schaller,
  • Vanessa Wood,
  • Xijie Wang,
  • Jennifer A. Dionne,
  • Dmitri V. Talapin,
  • A. Paul Alivisatos,
  • Alberto Salleo,
  • Eran Rabani,
  • Aaron M. Lindenberg

DOI
https://doi.org/10.1038/s41467-021-22116-0
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 9

Abstract

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Charge trapping can lead to severe nonradiative losses in colloidal semiconductor nanocrystals (NCs). The authors report femtosecond electron diffraction measurements on photoexcited NCs to reveal atomic-scale insights into how localization of charges at trap sites induce surface deformations.