Quantum Path Interference and Multiple Electron Scattering in Soft X-Ray High-Order Harmonic Generation

Abstract

High-order harmonic generation is an important mechanism to generate coherent radiation in the few–100-eV spectral range with ultrashort laser pulses. Moreover, a closer inspection of the measured spectra provides unique information about the underlying physics and allows deriving guidelines for improvements. The long-range modulation of the spectral envelope is linked to phase matching, and we will show how to improve it with a double-pulse excitation scheme. Additionally, the spectrum contains only every fourth harmonic, which can be well explained by the quantum interference of multiple scattered electrons, and two dominant electron trajectories were selected by X-ray parametric interaction.

Keywords

• high harmonic generation
• nonlinear optics
• ultrafast optics