A Bayesian Framework to Quantify Uncertainty in Aerosol Optical Model Selection Applied to TROPOMI Measurements

Abstract

This article presents a method within a Bayesian framework for quantifying uncertainty in satellite aerosol remote sensing when retrieving aerosol optical depth (AOD). By using a Bayesian model averaging technique, we take into account uncertainty in aerosol optical model selection and also obtain a shared inference about AOD based on the best-fitting optical models. In particular, uncertainty caused by forward-model approximations has been taken into account in the AOD retrieval process to obtain a more realistic uncertainty estimate. We evaluated a model discrepancy, i.e., forward-model uncertainty, empirically by exploiting the residuals of model fits and using a Gaussian process to characterise the discrepancy. We illustrate the method with examples using observations from the TROPOspheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor satellite. We evaluated the results against ground-based remote sensing aerosol data from the Aerosol Robotic Network (AERONET).

Keywords

• aerosol retrieval
• model selection
• uncertainty
• Bayesian inference
• TROPOMI/S5P