Nature Communications (Aug 2018)
Field- and temperature-dependent quantum tunnelling of the magnetisation in a large barrier single-molecule magnet
Abstract
Understanding quantum tunnelling of the magnetisation in single-molecule magnets is crucial for their potential application in information storage. Here the authors conduct a field- and temperature-dependent study of the magnetisation dynamics of a dysprosium-based SMM, finding four distinct relaxation processes that dominate in different regimes.