First order phase transition between two centro-symmetric superradiant crystals

Abstract

We observe a structural phase transition between two configurations of a superradiant crystal by coupling a Bose-Einstein condensate to an optical cavity and applying imbalanced transverse pump fields. The transition can be interpreted as a transition between two nonpolar, centro-symmetric structures involving a change in polarization. We find that this first order phase transition is accompanied by transient dynamics of the order parameter which we measure in real time. The phase transition and the excitation spectrum can be derived from a microscopic Hamiltonian, in quantitative agreement with our experimental data.