Atmospheric Chemistry and Physics (May 2019)
Rapid ice aggregation process revealed through triple-wavelength Doppler spectrum radar analysis
Abstract
We have identified a region of an ice cloud where a sharp transition of dual-wavelength ratio occurs at a fixed height for longer than 20 min. In this paper we provide evidence that rapid aggregation of ice particles occurred in this region, creating large particles. This evidence comes from triple-wavelength Doppler spectrum radar data that were fortuitously being collected. Through quantitative comparison of the Doppler spectra from the three radars we are able to estimate the ice particle size distribution (of particles larger than 0.75 mm) at different heights in the cloud. This allows us to investigate the evolution of the ice particle size distribution and determine whether the evolution is consistent with aggregation, riming or vapour deposition. The newly developed method allows us to isolate the signal from the larger (non-Rayleigh scattering) particles in the distribution. Therefore, a particle size distribution retrieval is possible in areas of the cloud where the dual-wavelength ratio method would fail because the bulk dual-wavelength ratio value is too close to zero. The ice particles grow rapidly from a maximum size of 0.75 to 5 mm while falling less than 500 m in under 10 min. This rapid growth is shown to agree well with theoretical estimates of aggregation, with aggregation efficiency being approximately 0.7, and is inconsistent with other growth processes, e.g. growth by vapour deposition or riming. The aggregation occurs in the middle of the cloud and is not present throughout the entire lifetime of the cloud. However, the layer of rapid aggregation is very well defined at a constant height, where the temperature is −15 ∘C and lasts for at least 20 min (approximate horizontal distance: 24 km). Immediately above this layer, the radar Doppler spectrum is bi-modal, which signals the formation of new small ice particles at that height. We suggest that these newly formed particles, at approximately −15 ∘C, grow dendritic arms, enabling them to easily interlock and accelerate the aggregation process. The large estimated aggregation efficiency in this cloud is consistent with recent laboratory studies for dendrites at this temperature.