Slow positron beam study on defects induced by Xe ions irridiation in matrix graphite of fuel elements

XU Hongxia; LIN Jun; ZHU Zhiyong; LIU Jiandang; GU Bingchuan; YE Bangjiao

doi:10.11889/j.0253-3219.2022.hjs.45.100204

He jishu (Oct 2022)

Slow positron beam study on defects induced by Xe ions irridiation in matrix graphite of fuel elements

XU Hongxia,
LIN Jun,
ZHU Zhiyong,
LIU Jiandang,
GU Bingchuan,
YE Bangjiao

Affiliations

XU Hongxia: Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China
LIN Jun: Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China
ZHU Zhiyong: Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China
LIU Jiandang: State Key Laboratory of Particle Detection and Electronics, University of Science and Technology of China, Hefei 230026, China
GU Bingchuan: State Key Laboratory of Particle Detection and Electronics, University of Science and Technology of China, Hefei 230026, China
YE Bangjiao: State Key Laboratory of Particle Detection and Electronics, University of Science and Technology of China, Hefei 230026, China

DOI: https://doi.org/10.11889/j.0253-3219.2022.hjs.45.100204
Journal volume & issue: Vol. 45, no. 10
pp. 100204 – 100204

Abstract

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Background The solid fuel thorium element molten salt reactors (MSR) have attracted more attention recent years. A3-3 graphite is chosen as the fuel matrix for MSR, thus its irradiation behavior and mechanical property is very important before the application. Purpose The study aims to observe the irradiation defects and hardness of A3-3 matrix graphite after ion irradiation by slow positron beam and nano-indentation, respectively. Methods The matrix graphite of fuel elements was irradiated with 1 MeV Xe ions to fluence of 5.8×1014 ions·cm-2 and 2.9×1015 ions·cm-2 respectively at room temperature. The slow positron beam and nano-indentation were employed to investigate the effect of Xe ions irradiation on vacancy defects and hardness of matrix graphite. The changes in irradiation induced defects distribution with depth and fluence were analyzed according to the obtained positron annihilation S parameters versus positron incidence energy or depth curves, compared to SRIM (Stopping and Range of Ions in Matter) calculation. Results Results from slow positron beam measurement show that 1 MeV Xe ions irradiation in matrix graphite introduces a damage layer with depth of about 600 nm, and the damage peak locates at about 250~350 nm in depth, consisted with SRIM simulation. The S parameters in irradiation samples increase significantly compared to virgin sample, which suggests that a high concentration of vacancy-type defects appeared within irradiation damage layer. In addition, the S parameters increase with the irradiation fluence, which shows that the concentration or size of vacancy-type defects increases. The nano-indentation results show that the hardness of irradiated graphite matrix is enhanced. Conclusions The enhanced hardness of A3-3 matrix graphite after ion irradiation is ascribed to the pinning of basal plane dislocation by the high concentration of vacancy type defects introduced by irradiation, consisted with the slow positron beam analysis. Slow positron beam is a very sensitive tool to study the irradiation defects.

Published in He jishu

ISSN: 0253-3219 (Print)
Publisher: Science Press
Country of publisher: China
LCC subjects: Technology: Electrical engineering. Electronics. Nuclear engineering: Nuclear engineering. Atomic power
Website: https://www.hjs.sinap.ac.cn/

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