Modulating oxygen coverage of Ti3C2Tx MXenes to boost catalytic activity for HCOOH dehydrogenation

Tingting Hou; Qiquan Luo; Qi Li; Hualu Zu; Peixin Cui; Siwei Chen; Yue Lin; Jiajia Chen; Xusheng Zheng; Wenkun Zhu; Shuquan Liang; Jinlong Yang; Liangbing Wang

doi:10.1038/s41467-020-18091-7

Nature Communications (Aug 2020)

Modulating oxygen coverage of Ti3C2Tx MXenes to boost catalytic activity for HCOOH dehydrogenation

Tingting Hou,
Qiquan Luo,
Qi Li,
Hualu Zu,
Peixin Cui,
Siwei Chen,
Yue Lin,
Jiajia Chen,
Xusheng Zheng,
Wenkun Zhu,
Shuquan Liang,
Jinlong Yang,
Liangbing Wang

Affiliations

Tingting Hou: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University
Qiquan Luo: Institutes of Physical Science and Information Technology, Anhui University
Qi Li: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University
Hualu Zu: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University
Peixin Cui: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, the Chinese Academy of Sciences
Siwei Chen: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University
Yue Lin: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Jiajia Chen: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Xusheng Zheng: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Wenkun Zhu: State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology
Shuquan Liang: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University
Jinlong Yang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Liangbing Wang: State Key Laboratory for Powder Metallurgy, Key Laboratory of Electronic Packing and Advanced Functional Materials of Hunan Province, School of Materials Science and Engineering, Central South University

DOI: https://doi.org/10.1038/s41467-020-18091-7
Journal volume & issue: Vol. 11, no. 1
pp. 1 – 11

Abstract

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Developing non-noble-metal heterogeneous catalysts with high efficiency in HCOOH dehydrogenation is significant for the acquisition of hydrogen, but remains a great challenge. Here, the authors modulate oxygen coverage of Ti3C2Tx MXenes to boost the catalytic activity toward HCOOH dehydrogenation.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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