npj Quantum Materials (Mar 2021)
Classical magnetic vortex liquid and large thermal Hall conductivity in frustrated magnets with bond-dependent interactions
Abstract
Abstract Recently, the observation of large thermal Hall conductivities in correlated insulators with no apparent broken symmetry has generated immense interest and debates on the underlying ground states. Here, considering frustrated magnets with bond-dependent interactions, which are realized in the so-called Kitaev materials, we theoretically demonstrate that a large thermal Hall conductivity can originate from a classical ground state without any magnetic order. We discover a liquid state of magnetic vortices, which are inhomogeneous spin textures embedded in the background of polarized spins, under out-of-plane magnetic fields. In the classical regime, different configurations of vortices form an effectively degenerate manifold. We study the static and dynamical properties of the magnetic vortex liquid state at zero and finite temperatures. In particular, we show that the spin excitation spectrum resembles a continuum of nearly flat Chern bands, which ultimately leads to a large thermal Hall conductivity. Possible connections to experiments are discussed.