Quantum interference directed chiral raman scattering in two-dimensional enantiomers

Shishu Zhang; Jianqi Huang; Yue Yu; Shanshan Wang; Teng Yang; Zhidong Zhang; Lianming Tong; Jin Zhang

doi:10.1038/s41467-022-28877-6

Nature Communications (Mar 2022)

Quantum interference directed chiral raman scattering in two-dimensional enantiomers

Shishu Zhang,
Jianqi Huang,
Yue Yu,
Shanshan Wang,
Teng Yang,
Zhidong Zhang,
Lianming Tong,
Jin Zhang

Affiliations

Shishu Zhang: Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University
Jianqi Huang: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Yue Yu: Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University
Shanshan Wang: Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University
Teng Yang: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Zhidong Zhang: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Lianming Tong: Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University
Jin Zhang: Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University

DOI: https://doi.org/10.1038/s41467-022-28877-6
Journal volume & issue: Vol. 13, no. 1
pp. 1 – 7

Abstract

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Quantum interference among elementary Raman processes has only been observed in few materials under specific excitation configurations. Here, the authors show that quantum interference can lead to significant chiral Raman response in a monolayer material of transitional metal dichalcogenide with triclinic symmetry.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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