Emissions and Atmospheric Dry and Wet Deposition of Trace Metals from Natural and Anthropogenic Sources in Mainland China
Shenglan Jiang,
Xuyang Dong,
Zimin Han,
Junri Zhao,
Yan Zhang
Affiliations
Shenglan Jiang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
Xuyang Dong
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
Zimin Han
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
Junri Zhao
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
Yan Zhang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
Trace metals from natural and anthropogenic sources impact the atmospheric environment and enter the soil through dry and wet atmospheric deposition, ultimately affecting human health. In this study, we established an emission inventory of Pb, As, Cr, and Cd in East Asia (80° E–140° E, 15° N–50° N) for the year 2017, including dust and anthropogenic sources from both land and marine. We modified the Community Multiscale Air Quality (CMAQ) model to provide gridded data on concentrations, as well as dry and wet atmospheric deposition fluxes of metals, with a focus on mainland China. The emissions of Pb, As, Cr, and Cd in East Asia were 19,253, 3415, 3332, and 9379 tons, respectively, in 2017, with 55%, 69%, 25%, and 58% distributed in the fine mode. The spatial distribution of atmospheric concentrations and dry deposition of trace metals was similar to that of emissions, while the spatial distribution of precipitation-related wet deposition was further east and greater in the south than in the north. In mainland China, the average bulk-deposition fluxes of Pb, As, Cr, and Cd were 1036.5, 170.3, 465.9, and 185.0 μg·m−2·year−1, respectively. Our study provides gridded data on trace metals in mainland China, which can be used for assessing air quality, human exposure risks, and metal inputs to soils.
