Nano-Micro Letters (Apr 2024)

Compliant Iontronic Triboelectric Gels with Phase-Locked Structure Enabled by Competitive Hydrogen Bonding

  • Guoli Du,
  • Yuzheng Shao,
  • Bin Luo,
  • Tao Liu,
  • Jiamin Zhao,
  • Ying Qin,
  • Jinlong Wang,
  • Song Zhang,
  • Mingchao Chi,
  • Cong Gao,
  • Yanhua Liu,
  • Chenchen Cai,
  • Shuangfei Wang,
  • Shuangxi Nie

DOI
https://doi.org/10.1007/s40820-024-01387-4
Journal volume & issue
Vol. 16, no. 1
pp. 1 – 15

Abstract

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Highlights A bionic phase-locked structure-inspired iontronic triboelectric gel is proposed with good mechanical compliance for wearable haptic sensing applications. Competitive hydrogen bonding systems are constructed through polymer-solvent-nonsolvent interactions, and regeneration of polymers with weak hydrogen bond donors triggers controlled phase separation. Self-powered haptic skin constructed with iontronic triboelectric gel has a modulus (150.6 kPa) and stretchability (> 400%) similar to that of the human body, enabling fidelity transmission of haptic signals and precise recognition of sensing objects.

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