Physical Review Research (Jan 2025)

Radiative decay of the ^{229m}Th nuclear clock isomer in different host materials

  • S. V. Pineda,
  • P. Chhetri,
  • S. Bara,
  • Y. Elskens,
  • S. Casci,
  • A. N. Alexandrova,
  • M. Au,
  • M. Athanasakis-Kaklamanakis,
  • M. Bartokos,
  • K. Beeks,
  • C. Bernerd,
  • A. Claessens,
  • K. Chrysalidis,
  • T. E. Cocolios,
  • J. G. Correia,
  • H. De Witte,
  • R. Elwell,
  • R. Ferrer,
  • R. Heinke,
  • E. R. Hudson,
  • F. Ivandikov,
  • Yu. Kudryavtsev,
  • U. Köster,
  • S. Kraemer,
  • M. Laatiaoui,
  • R. Lica,
  • C. Merckling,
  • I. Morawetz,
  • H. W. T. Morgan,
  • D. Moritz,
  • L. M. C. Pereira,
  • S. Raeder,
  • S. Rothe,
  • F. Schaden,
  • K. Scharl,
  • T. Schumm,
  • S. Stegemann,
  • J. Terhune,
  • P. G. Thirolf,
  • S. M. Tunhuma,
  • P. Van Den Bergh,
  • P. Van Duppen,
  • A. Vantomme,
  • U. Wahl,
  • Z. Yue

DOI
https://doi.org/10.1103/PhysRevResearch.7.013052
Journal volume & issue
Vol. 7, no. 1
p. 013052

Abstract

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A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the ^{229m}Th nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons and the number of ^{229m}Th embedded are determined for single crystalline CaF_{2}, MgF_{2}, LiSrAlF_{6}, AlN, and amorphous SiO_{2}. For the latter two materials, no radiative decay signal was observed and an upper limit of the ratio is reported. The radiative decay wavelength was determined in LiSrAlF_{6} and CaF_{2}, reducing its uncertainty by a factor of 2.5 relative to our previous measurement. This value is in agreement with the recently reported improved values from laser excitation.